| description abstract | Infrared measurements can be used to obtain quantitative information on cloud microphysics, including cloud composition (ice, liquid water, ash, dust, etc.), with the advantage that the measurements are independent of solar zenith angle. As such, infrared brightness temperatures (BT) and brightness temperature differences (BTD) have been used extensively in quantitative remote sensing applications for inferring cloud composition. In this study it is shown that BTDs are fundamentally limited and that a more physically based infrared approach can lead to significant increases in sensitivity to cloud microphysics, especially for optically thin clouds. In lieu of BTDs, a derived radiative parameter ?, which is directly related to particle size, habit, and composition, is used. Although the concept of effective absorption optical depth ratios ? has been around since the mid-1980s, this is the first study to explore the use of ? for inferring cloud composition in the total absence of cloud vertical boundary information. The results showed that, even in the absence of cloud vertical boundary information, one could significantly increase the sensitivity to cloud microphysics by converting the measured radiances to effective emissivity and constructing effective absorption optical depth ratios from a pair of spectral emissivities in the 8?12-?m ?window.? This increase in sensitivity to cloud microphysics is relative to BTDs constructed from the same spectral pairs. In this article, the focus is on describing the physical concepts (which can be applied to narrowband or hyperspectral infrared measurements) used in constructing the ? data space. | |
