Analytical Solutions to the Stochastic Kinetic Equation for Liquid and Ice Particle Size Spectra. Part I: Small-Size Fraction

Abstract

The kinetic equation of stochastic condensation for cloud drop size spectra is extended to account for crystalline clouds and also to include the accretion?aggregation process. The size spectra are separated into small and large size fractions that correspond to cloud drops (ice) and rain (snow). In Part I of this two-part paper, analytical solutions are derived for the small-size fractions of the spectra that correspond to cloud drops and cloud ice particles that can be identified with cloud liquid water or cloud ice water content, and used in bulk microphysical schemes employed in cloud and climate models. Solutions for the small-size fraction have the form of generalized gamma distributions. Simple analytical expressions are found for parameters of the gamma distributions that are functions of quantities that are available in cloud and climate models: liquid or ice water content and its vertical gradient, mean particle radius or concentration, and supersaturation or vertical velocities. Equations for the gamma distribution parameters provide an explanation of the dependence of the observed spectra on atmospheric dynamics, cloud temperature, and cloud liquid water or ice water content. The results are illustrated with example calculations for a crystalline cloud. The analytical solutions and expressions for the parameters presented here can be used for parameterization of the small-size fraction size spectra in liquid and crystalline clouds and related quantities (e.g., optical properties, lidar, and radar reflectivities).