Impacts of Meteorological Conditions, Aerosol Radiative Feedbacks, and Emission Reduction Scenarios on the Coastal Haze Episodes in Southeastern China in December 2013

Abstract

ujian Province in southeastern coastal China is a relatively clean region with low emissions, as its high altitude isolates it from the rest of the country. However, the region experienced haze episodes on 3?14 December 2013. The authors performed simulations using the Weather Research and Forecasting Model coupled with chemistry (WRF-Chem) to examine the impacts of meteorological conditions, aerosol radiative feedbacks (ARFs; including aerosol direct and nearly first indirect effect), and internal and external emissions reduction scenarios on particulate matter smaller than 2.5 ?m (PM2.5) concentrations. To the best of the authors? knowledge, this is the first time the WRF-Chem model has been used to study air quality in this region. The model reasonably reproduced the meteorological conditions and PM2.5 concentrations. The analysis demonstrated that the highest-PM2.5 event was associated with a cold surge that promoted the impingement of northern pollutants on the region, and PM2.5 concentrations were sensitive to the emissions from the Yangtze River delta (16.6%) and the North China Plain (12.1%). This suggests that efforts toward coastal air quality improvement require regional cooperation to reduce emissions. Noticeably, ARFs were unlikely to increase PM2.5 concentrations in the coastal region, which was in contrast to the case in northern China. ARFs induced strong clean wind anomalies in the coastal region and also lowered the inland planetary boundary layer, which enhanced the blocking of northern pollutants crossing the high terrain in the north of Fujian Province. This indicates that ARFs tend to weaken the haze intensity in the southeastern coastal region.