Evaporation of Nonequilibrium Raindrops as a Fog Formation Mechanism

Abstract

To gain insights into the poorly understood phenomenon of precipitation fog, this study assesses the evaporation of freely falling drops departing from equilibrium as a possible contributing factor to fog formation in rainy conditions. The study is based on simulations performed with a microphysical column model describing the evolution of the temperature and mass of evaporating raindrops within a Lagrangian reference frame. Equilibrium defines a state where the latent heat loss of an evaporating drop is balanced by the sensible heat flux from the ambient air, hence defining a steady-state drop temperature. Model results show that the assumption of equilibrium leads to small but significant errors in calculated precipitation evaporation rates for drops falling in continuously varying ambient near-saturated or saturated conditions. Departure from equilibrium depends on the magnitude of the vertical gradients of the ambient temperature and moisture as well as the drop-size-dependent terminal velocity. Contrasting patterns of behavior occur depending on the stratification of the atmosphere. Raindrops falling in inversion layers remain warmer than the equilibrium temperature and lead to enhanced moistening, with supersaturation achieved when evaporation proceeds in saturated inversions. Dehydration occurs in layers with temperature and water vapor increasing with height due to the vapor flux from the environment to the colder drops. These contrasts are not represented when equilibrium is assumed. The role of nonequilibrium raindrop evaporation in fog occurrences is further emphasized with simulations of a case study characterized by fog forming under light rain falling in a developing frontal inversion. Good agreement is obtained between fog water content observations and simulations representing only the effects of rainfall evaporation. This study demonstrates the need to take into account the nonequilibrium state of falling raindrops for a proper representation of an important mechanism contributing to precipitation fog occurrences.